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Journal Articles

Investigation of hydrogen superoxide adsorption during ORR on Pt/C catalyst in acidic solution for PEFC by ${it in-situ}$ high energy resolution XAFS

Yamamoto, Naoki*; Matsumura, Daiju; Hagihara, Yuto*; Tanaka, Kei*; Hasegawa, Yuta*; Ishii, Kenji*; Tanaka, Hirohisa*

Journal of Power Sources, 557, p.232508_1 - 232508_10, 2023/02

 Times Cited Count:2 Percentile:29.01(Chemistry, Physical)

Journal Articles

The First application of a Gd$$_{3}$$Al$$_{2}$$Ga$$_{3}$$O$$_{12}$$:Ce single-crystal scintillator to neutron radiography

Isegawa, Kazuhisa; Setoyama, Daigo*; Kimura, Hidehiko*; Shinohara, Takenao

Journal of Imaging (Internet), 7(11), p.232_1 - 232_9, 2021/11

Neutron radiography is regarded as complementary to X-ray radiography in terms of transmittance through materials, but its spatial resolution is still insufficient. In order to achieve higher resolution in neutron imaging, several approaches have been adopted such as optical magnification and event centroiding, and the authors focused on modification of the scintillator in this paper. A Gd$$_{3}$$Al$$_{2}$$Ga$$_{3}$$O$$_{12}$$:Ce single-crystal scintillator was applied to neutron radiography for the first time and was achieved a spatial resolution of 10.5 micrometers. The results indicate that this material can be a powerful candidate for a new neutron scintillator providing a resolution in micrometer order by optimizing the optical system and increasing the scintillator luminosity.

Journal Articles

Lattice dynamics in FeSe via inelastic X-ray scattering and first-principles calculations

Murai, Naoki; Fukuda, Tatsuo; Nakajima, Masamichi*; Kawamura, Mitsuaki*; Ishikawa, Daisuke*; Tajima, Setsuko*; Baron, A. Q. R.*

Physical Review B, 101(3), p.035126_1 - 035126_6, 2020/01

 Times Cited Count:5 Percentile:33.01(Materials Science, Multidisciplinary)

We report an inelastic X-ray scattering investigation of phonons in FeSe superconductor. Comparing the experimental phonon dispersion with density functional theory (DFT) calculations in the non-magnetic state, we found a significant disagreement between them. A better overall agreement was obtained by allowing for spin-polarization in DFT calculations, despite the absence of magnetic order in FeSe. This calculation gives a realistic approximation, at DFT level, of the disordered paramagnetic state of FeSe, in which strong spin fluctuations are present.

Journal Articles

A Submillimeter spatial resolution scintillation detector for time-of-flight neutron diffraction imaging

Nakamura, Tatsuya; Kawasaki, Takuro; To, Kentaro; Tsutsui, Noriaki; Ebine, Masumi; Birumachi, Atsushi; Sakasai, Kaoru

Proceedings of 2018 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2018) (Internet), 3 Pages, 2019/10

A two-dimensional scintillation neutron detector with a submillimeter spatial resolution was developed for pulsed neutron diffraction imaging at the J-PARC MLF. The detector comprised the thin, single ZnS/$$^{6}$$LiF scintillator screen coupled with the crossed wavelength-shifting fiber array for light collection. For a high spatial resolution, the wavelength shifting fibers with diameter of 0.1 mm were used them for assembling the detector. The prototype detector that has a neutron-sensitive area of 24 $$times$$ 24 mm$$^{2}$$ exhibited a spatial resolution of 0.20$$pm$$0.06 mm and 0.16$$pm$$0.06 mm for x and y directions, respectively. The detector had a detection efficiency of 7$$%$$ for thermal neutrons with a $$^{60}$$Co $$gamma$$-ray sensitivity in the order of 10$$^{-6}$$. In this paper detailed detector design is presented together with experimental results using the pulsed neutron beam.

Journal Articles

Electrochemical adsorption on Pt nanoparticles in alkaline solution observed using in situ high energy resolution X-ray absorption spectroscopy

Kusano, Shogo*; Matsumura, Daiju; Ishii, Kenji*; Tanaka, Hirohisa*; Mizuki, Junichiro*

Nanomaterials (Internet), 9(4), p.642_1 - 642_14, 2019/04

 Times Cited Count:7 Percentile:37.59(Chemistry, Multidisciplinary)

Journal Articles

Effect of water for the oxygen adsorption on surface of PtCo catalysts

Cui, Y.-T.*; Harada, Yoshihisa*; Niwa, Hideharu*; Oshima, Masaharu*; Hatanaka, Tatsuya*; Nakamura, Naoki*; Ando, Masaki*; Yoshida, Toshihiko*; Ishii, Kenji*; Matsumura, Daiju

NanotechJapan Bulletin (Internet), 11(4), 6 Pages, 2018/08

no abstracts in English

Journal Articles

LES studies for predicting plume concentrations around nuclear facilities using an overlapping technique

Nakayama, Hiromasa; Takemi, Tetsuya*

Proceedings of 18th International Conference on Harmonisation within Atmospheric Dispersion Modelling for Regulatory Purposes (HARMO-18) (USB Flash Drive), p.843 - 847, 2017/10

We have attempted to develop a practical and quick local-scale atmospheric dispersion calculation method using an overlapping technique for plume concentration distributions in an emergency response to nuclear accidents. In order to evaluate the overlapping approach, we performed LESs of turbulent flows and plume dispersion under varying mean wind directions using the meteorological data as the model input. When compared with the simulated results under the real meteorological condition, it is shown that the concentration distribution patterns are reasonably simulated by the overlapping method. It can be concluded that the atmospheric dispersion calculation method using the overlapping technique has potential performance for emergency responses to nuclear accidents.

Journal Articles

Solid parahydrogen and ESR

Kumada, Takayuki

Kagaku No Yoten Shirizu, 20, P. 71, 2017/06

no abstracts in English

Journal Articles

Wetting induced oxidation of Pt-based nano catalysts revealed by ${{it in situ}}$ high energy resolution X-ray absorption spectroscopy

Cui, Y.-T.*; Harada, Yoshihisa*; Niwa, Hideharu*; Hatanaka, Tatsuya*; Nakamura, Naoki*; Ando, Masaki*; Yoshida, Toshihiko*; Ishii, Kenji*; Matsumura, Daiju; Oji, Hiroshi*; et al.

Scientific Reports (Internet), 7(1), p.1482_1 - 1482_8, 2017/05

 Times Cited Count:19 Percentile:49.58(Multidisciplinary Sciences)

Journal Articles

Development of micro-structured fluorescent plates for high-resolution imaging

Sakai, Takuro; Yasuda, Ryo; Iikura, Hiroshi; Matsubayashi, Masahito

JPS Conference Proceedings (Internet), 11, p.020005_1 - 020005_6, 2016/11

Journal Articles

X-ray backscattering study of crystal lattice distortion in hidden order of URu$$_2$$Si$$_2$$

Tabata, Chihiro*; Inami, Toshiya; Michimura, Shinji*; Yokoyama, Makoto*; Hidaka, Hiroyuki*; Yanagisawa, Tatsuya*; Amitsuka, Hiroshi*

Philosophical Magazine, 94(32-33), p.3691 - 3701, 2014/00

 Times Cited Count:16 Percentile:57.9(Materials Science, Multidisciplinary)

Journal Articles

XAS and XPS combined analysis using high-resolution and high-flux soft X-ray from synchrotron radiation

Matsubayashi, Nobuyuki*; Tanaka, Tomoaki*; Imamura, Motoyasu*; Shimada, Hiromichi*; Saito, Takeru

Analytical Sciences (CD-ROM), 17(Suppl.), p.119 - 121, 2002/03

no abstracts in English

Journal Articles

High-resolution electron spin resonance spectroscopy of ethyl radicals in solid parahydrogen

Kumada, Takayuki; Kumagai, Jun*; Miyazaki, Tetsuo*

Journal of Chemical Physics, 114(22), p.10024 - 10030, 2001/06

 Times Cited Count:14 Percentile:41.27(Chemistry, Physical)

no abstracts in English

Journal Articles

High-resolution ESR spectroscopy using solid parahydrogen matrix

Kumada, Takayuki

Hoshasen Kagaku, 2001(71), p.43 - 47, 2001/03

no abstracts in English

JAEA Reports

A study on improvements in accuracy of nuclear data measurements using $$gamma$$-ray spectroscopic methods

Furutaka, Kazuyoshi

JNC TN8400 2000-028, 70 Pages, 2000/10

JNC-TN8400-2000-028.pdf:1.71MB

This report describes the study done by the author as a postdoctoral research associate at Japan Nuclear Cycle Development Institute. This report is divided into two parts: improvements in accuracy in determination of thermal neutron capture cross sections, and improvements in accuracy of photo-nuclear absorption cross section measurements using the HHS. (1)In the measurements of thermal neutron capture cross sections using an activation method, accuracies of the final results attained are limited by (1) accuracy of $$gamma$$-ray peak detection efficiencies, and (2) accuracies of $$gamma$$-ray emission probabilities. In this study; to determine thermal neutron capture cross sections more accurately, the following researches have been done using a newly developed three-dimensional coincidence measurement system: (1)accurate determination of $$gamma$$-ray standard sources using a $$gamma$$-$$gamma$$ coincidence method, for precise calibration of $$gamma$$-ray peak detection efficiency, and (2) development of a $$beta$$-$$gamma$$ coincidence measurement system using a plastic scintillation detector as a $$beta$$-ray detector, for the determination of $$gamma$$-ray emission probabilities of short-lived nuclides, and measurement of $$gamma$$-ray emission probabilities of $$^{100}$$Tc nuclide using the coincidence system. (2)To transform radioactive nuclides with small thermal neutron capture cross sections, use of photonuclear absorption reaction has been suggested. In order to transform these nuclides efficiently using the reaction, one has to know detailed behavior of the photo-absorption cross sections. In this study, a Monte-Carlo simulation code has been used to create a standard set of $$gamma$$-ray response functions of the high-resolution high-energy spectrometer (HHS), to enable reliable analyses of the data obtained by the spectrometer.

Journal Articles

A Focusing monochromator of neutron diffractometer for residual stress analysis (RESA)

Minakawa, Nobuaki; Morii, Yukio; Shimojo, Yutaka

Proceedings of 6th International Conference on Residual Stressess (ICRS-6), Vol.2, p.1107 - 1111, 2000/07

no abstracts in English

Journal Articles

Probing bulk states of correlated electron systems by high-resolution resonance photoemission

Sekiyama, Akira*; Iwasaki, T.*; Matsuda, K.*; Saito, Yuji; Onuki, Yoshichika*; Suga, Shigemasa*

Nature, 403(6768), p.396 - 398, 2000/01

 Times Cited Count:255 Percentile:98.93(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

The Spectral profile of the He I singlet line (667.82nm) emitted from the divertor region of JT-60U

Kubo, Hirotaka; Takenaga, Hidenobu; Kumagai, Akira*; Higashijima, Satoru; Suzuki, Shingo*; Sugie, Tatsuo; Sakasai, Akira; Itami, Kiyoshi

Plasma Physics and Controlled Fusion, 41(6), p.747 - 757, 1999/00

 Times Cited Count:20 Percentile:55.12(Physics, Fluids & Plasmas)

no abstracts in English

JAEA Reports

Technical development and operation of TV Thomson scattering system on JFT-2M tokamak

; Yamauchi, Toshihiko; *; *; Yoshida, Hidetoshi; Kozawa, Teruo; *; *; D.Dimock*; B.LeBlanc*; et al.

JAERI-Tech 98-048, 49 Pages, 1998/10

JAERI-Tech-98-048.pdf:2.16MB

no abstracts in English

Journal Articles

Twin helical undulator beamline for soft X-ray spectroscopy at SPring-8

Saito, Yuji; Nakatani, Takeshi*; Matsushita, T.*; Miyahara, Tsuneaki*; Fujisawa, M.*; *; *; *; *; *; et al.

Journal of Synchrotron Radiation, 5, p.542 - 544, 1998/00

 Times Cited Count:62 Percentile:94.44(Instruments & Instrumentation)

no abstracts in English

42 (Records 1-20 displayed on this page)